To put it simply, story follows the live of Imperius and Tyrael, but other members of Angiris Council can be counted as main characters - same way as Rias Gremory and his peerage's members.
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Imperius is archangel of Valor, who leads the angiris council in broad daylight, while its actual leader, Malthael, stays in the shadows. Imperius shines both in abilities to lead as well as mighty warrior. He is, as they could say: "The one who slays the prime evil.
Imperius wields Solarion, the spear of Valor, and thus lives by his name. In High Heavens, his corresponding domain is Halls of Valor.
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Tyrael is Archangel of Justice, and has close friendship with Imperius. As archangel of Justice, Tyrael has straightforward sense of justice and he is somewhat "Maverick" of the Angiris Council. He is impartial dispenser of justice, and for his aspect, he wields El'druin, the sword of justice. Tyrael corresponding domain High Heavens is Courts of Justice.
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Auriel is the Voice of Reason and pillar of diplomacy in the Council and its only female member. She is also closest to Itherael. Auriel is compassionate, but she's willing to fight if its necessary. She wields Al'maiesh, the cord of hope. Her corresponding domain in High Heavens is Gardens of Hope.
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Itherael is Archangel of fate. he is mostly aloof, but is still closest to Auriel. He also reads Talus'ar, the Scroll of Fate, which allows Archangels foresee future events. His corresponding domain is Library of Fate.
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Malthael is archangel and his aspect is actually Wisdom, though he also acts angel of Death in times of war. He is the true leader of the Angiris council, and works in the shadows while outsiders focus their mind to Imperius. He offers knowledge to all members of Angiris Council and when it's needed, outsiders too.
As angel of Death he is weaponized with two sickles, but as the archangel of Wisdom, he wields Chalad'ar, the Chalice of Wisdom. In High Heavens, his corresponding domain is Pools of Wsdom.
